[Adsorption Characteristics of Biochar on Heavy Metals (Pb and Zn) in Soil].
Identifieur interne : 001121 ( Main/Exploration ); précédent : 001120; suivant : 001122[Adsorption Characteristics of Biochar on Heavy Metals (Pb and Zn) in Soil].
Auteurs : Hong Wang [République populaire de Chine] ; Wen Xia [République populaire de Chine] ; Ping Lu [République populaire de Chine] ; Yu-Wei Bu [République populaire de Chine] ; Hao Yang [République populaire de Chine]Source :
- Huan jing ke xue= Huanjing kexue [ 0250-3301 ] ; 2017.
Descripteurs français
- KwdFr :
- MESH :
- composition chimique : Charbon de bois, Plomb, Polluants du sol, Zinc.
- Adsorption, Chine, Eichhornia, Mine, Populus, Sol, Zea mays.
English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Charcoal, Lead, Soil Pollutants, Zinc.
- Adsorption, China, Eichhornia, Mining, Populus, Soil, Zea mays.
Abstract
Three types of biochars, poplar branch biochar (PBC), water hyacinth biochar (WHC), and corn straw biochar (CSC), were prepared in a fixed-bed pyrolyzer at different pyrolysis temperatures (300-700℃). The effects of biochar species, pyrolysis temperature, and biochar addition on adsorption characteristics of typical heavy metals (HMs) such as Pb and Zn in vegetable soil (collected from a lead-zinc-silver mining area, Nanjing, China) were investigated. The adsorption mechanism of biochar on HMs was discussed based on the analyses of pore structure, XRD, and FTIR of biochars. WHC biochar showed the best adsorption ability at the same experimental conditions with adsorption efficiencies on Zn and Pb of 21.83% and 44.57%, respectively. The relative adsorption capacities of Zn and Pb were 227.65 μg·g-1 and 363.76 μg·g-1 at the pyrolysis temperature of 500℃ and biochar addition of 5%. The adsorption efficiency of biochar on HMs in soil increased gradually with increasing pyrolysis temperature. WHC biochars prepared at 500℃ and 700℃ had similar adsorption capacities on Zn and Pb in soil indicating that the moderate pyrolysis may be a good choice for WHC with better physicochemical properties. Increasing the amount of WHC addition benefits the adsorption efficiency of HMs in soil, but does not increase the adsorption capacity. The adsorption efficiency of Pb in soil reaches 93.93% by adding 10% of WHC into the soil sample. The combined analyses based on the physicochemical properties of biochar and the results of soil HMs adsorption experiments suggest that ion exchange and complexation are prevailing mechanisms of the remediation of HM-contaminated soil by WHC biochars.
DOI: 10.13227/j.hjkx.201701171
PubMed: 29965278
Affiliations:
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Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042</wicri:regionArea><wicri:noRegion>Nanjing 210042</wicri:noRegion></affiliation></author><author><name sortKey="Lu, Ping" sort="Lu, Ping" uniqKey="Lu P" first="Ping" last="Lu">Ping Lu</name><affiliation wicri:level="1"><nlm:affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, 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Wen" sort="Xia, Wen" uniqKey="Xia W" first="Wen" last="Xia">Wen Xia</name><affiliation wicri:level="1"><nlm:affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042</wicri:regionArea><wicri:noRegion>Nanjing 210042</wicri:noRegion></affiliation></author><author><name sortKey="Lu, Ping" sort="Lu, Ping" uniqKey="Lu P" first="Ping" last="Lu">Ping Lu</name><affiliation wicri:level="1"><nlm:affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042</wicri:regionArea><wicri:noRegion>Nanjing 210042</wicri:noRegion></affiliation></author><author><name sortKey="Bu, Yu Wei" sort="Bu, Yu Wei" uniqKey="Bu Y" first="Yu-Wei" last="Bu">Yu-Wei Bu</name><affiliation wicri:level="1"><nlm:affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042</wicri:regionArea><wicri:noRegion>Nanjing 210042</wicri:noRegion></affiliation></author><author><name sortKey="Yang, Hao" sort="Yang, Hao" uniqKey="Yang H" first="Hao" last="Yang">Hao Yang</name><affiliation wicri:level="1"><nlm:affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042</wicri:regionArea><wicri:noRegion>Nanjing 210042</wicri:noRegion></affiliation></author></analytic><series><title level="j">Huan jing ke xue= Huanjing kexue</title><idno type="ISSN">0250-3301</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Adsorption (MeSH)</term><term>Charcoal (chemistry)</term><term>China (MeSH)</term><term>Eichhornia (MeSH)</term><term>Lead (chemistry)</term><term>Mining (MeSH)</term><term>Populus (MeSH)</term><term>Soil (MeSH)</term><term>Soil Pollutants (chemistry)</term><term>Zea mays (MeSH)</term><term>Zinc (chemistry)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Adsorption (MeSH)</term><term>Charbon de bois (composition chimique)</term><term>Chine (MeSH)</term><term>Eichhornia (MeSH)</term><term>Mine (MeSH)</term><term>Plomb (composition chimique)</term><term>Polluants du sol (composition chimique)</term><term>Populus (MeSH)</term><term>Sol (MeSH)</term><term>Zea mays (MeSH)</term><term>Zinc (composition chimique)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Charcoal</term><term>Lead</term><term>Soil Pollutants</term><term>Zinc</term></keywords><keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Charbon de bois</term><term>Plomb</term><term>Polluants du sol</term><term>Zinc</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Adsorption</term><term>China</term><term>Eichhornia</term><term>Mining</term><term>Populus</term><term>Soil</term><term>Zea mays</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Adsorption</term><term>Chine</term><term>Eichhornia</term><term>Mine</term><term>Populus</term><term>Sol</term><term>Zea mays</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Three types of biochars, poplar branch biochar (PBC), water hyacinth biochar (WHC), and corn straw biochar (CSC), were prepared in a fixed-bed pyrolyzer at different pyrolysis temperatures (300-700℃). The effects of biochar species, pyrolysis temperature, and biochar addition on adsorption characteristics of typical heavy metals (HMs) such as Pb and Zn in vegetable soil (collected from a lead-zinc-silver mining area, Nanjing, China) were investigated. The adsorption mechanism of biochar on HMs was discussed based on the analyses of pore structure, XRD, and FTIR of biochars. WHC biochar showed the best adsorption ability at the same experimental conditions with adsorption efficiencies on Zn and Pb of 21.83% and 44.57%, respectively. The relative adsorption capacities of Zn and Pb were 227.65 μg·g<sup>-1</sup> and 363.76 μg·g<sup>-1</sup> at the pyrolysis temperature of 500℃ and biochar addition of 5%. The adsorption efficiency of biochar on HMs in soil increased gradually with increasing pyrolysis temperature. WHC biochars prepared at 500℃ and 700℃ had similar adsorption capacities on Zn and Pb in soil indicating that the moderate pyrolysis may be a good choice for WHC with better physicochemical properties. Increasing the amount of WHC addition benefits the adsorption efficiency of HMs in soil, but does not increase the adsorption capacity. The adsorption efficiency of Pb in soil reaches 93.93% by adding 10% of WHC into the soil sample. The combined analyses based on the physicochemical properties of biochar and the results of soil HMs adsorption experiments suggest that ion exchange and complexation are prevailing mechanisms of the remediation of HM-contaminated soil by WHC biochars.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Curated" Owner="NLM"><PMID Version="1">29965278</PMID><DateCompleted><Year>2018</Year><Month>12</Month><Day>11</Day></DateCompleted><DateRevised><Year>2018</Year><Month>12</Month><Day>11</Day></DateRevised><Article PubModel="Print"><Journal><ISSN IssnType="Print">0250-3301</ISSN><JournalIssue CitedMedium="Print"><Volume>38</Volume><Issue>9</Issue><PubDate><Year>2017</Year><Month>Sep</Month><Day>08</Day></PubDate></JournalIssue><Title>Huan jing ke xue= Huanjing kexue</Title><ISOAbbreviation>Huan Jing Ke Xue</ISOAbbreviation></Journal><ArticleTitle>[Adsorption Characteristics of Biochar on Heavy Metals (Pb and Zn) in Soil].</ArticleTitle><Pagination><MedlinePgn>3944-3952</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.13227/j.hjkx.201701171</ELocationID><Abstract><AbstractText>Three types of biochars, poplar branch biochar (PBC), water hyacinth biochar (WHC), and corn straw biochar (CSC), were prepared in a fixed-bed pyrolyzer at different pyrolysis temperatures (300-700℃). The effects of biochar species, pyrolysis temperature, and biochar addition on adsorption characteristics of typical heavy metals (HMs) such as Pb and Zn in vegetable soil (collected from a lead-zinc-silver mining area, Nanjing, China) were investigated. The adsorption mechanism of biochar on HMs was discussed based on the analyses of pore structure, XRD, and FTIR of biochars. WHC biochar showed the best adsorption ability at the same experimental conditions with adsorption efficiencies on Zn and Pb of 21.83% and 44.57%, respectively. The relative adsorption capacities of Zn and Pb were 227.65 μg·g<sup>-1</sup> and 363.76 μg·g<sup>-1</sup> at the pyrolysis temperature of 500℃ and biochar addition of 5%. The adsorption efficiency of biochar on HMs in soil increased gradually with increasing pyrolysis temperature. WHC biochars prepared at 500℃ and 700℃ had similar adsorption capacities on Zn and Pb in soil indicating that the moderate pyrolysis may be a good choice for WHC with better physicochemical properties. Increasing the amount of WHC addition benefits the adsorption efficiency of HMs in soil, but does not increase the adsorption capacity. The adsorption efficiency of Pb in soil reaches 93.93% by adding 10% of WHC into the soil sample. The combined analyses based on the physicochemical properties of biochar and the results of soil HMs adsorption experiments suggest that ion exchange and complexation are prevailing mechanisms of the remediation of HM-contaminated soil by WHC biochars.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Hong</ForeName><Initials>H</Initials><AffiliationInfo><Affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Xia</LastName><ForeName>Wen</ForeName><Initials>W</Initials><AffiliationInfo><Affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Lu</LastName><ForeName>Ping</ForeName><Initials>P</Initials><AffiliationInfo><Affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Bu</LastName><ForeName>Yu-Wei</ForeName><Initials>YW</Initials><AffiliationInfo><Affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yang</LastName><ForeName>Hao</ForeName><Initials>H</Initials><AffiliationInfo><Affiliation>Jiangsu Provincial Key Laboratory of Materials Cycling and Pollution Control, School of Energy and Mechanical Engineering, Nanjing Normal University, Nanjing 210042, China.</Affiliation></AffiliationInfo></Author></AuthorList><Language>chi</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList></Article><MedlineJournalInfo><Country>China</Country><MedlineTA>Huan Jing Ke Xue</MedlineTA><NlmUniqueID>8405344</NlmUniqueID><ISSNLinking>0250-3301</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D012987">Soil</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D012989">Soil Pollutants</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="C540010">biochar</NameOfSubstance></Chemical><Chemical><RegistryNumber>16291-96-6</RegistryNumber><NameOfSubstance UI="D002606">Charcoal</NameOfSubstance></Chemical><Chemical><RegistryNumber>2P299V784P</RegistryNumber><NameOfSubstance UI="D007854">Lead</NameOfSubstance></Chemical><Chemical><RegistryNumber>J41CSQ7QDS</RegistryNumber><NameOfSubstance UI="D015032">Zinc</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000327" MajorTopicYN="N">Adsorption</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002606" MajorTopicYN="N">Charcoal</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D002681" MajorTopicYN="N">China</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D031806" MajorTopicYN="N">Eichhornia</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D007854" MajorTopicYN="N">Lead</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D008906" MajorTopicYN="N">Mining</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D032107" MajorTopicYN="N">Populus</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D012987" MajorTopicYN="N">Soil</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D012989" MajorTopicYN="N">Soil Pollutants</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D003313" MajorTopicYN="N">Zea mays</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D015032" MajorTopicYN="N">Zinc</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Pb</Keyword><Keyword MajorTopicYN="N">Zn</Keyword><Keyword MajorTopicYN="N">adsorption characteristics</Keyword><Keyword MajorTopicYN="N">biochar</Keyword><Keyword MajorTopicYN="N">soil</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2018</Year><Month>7</Month><Day>3</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2018</Year><Month>7</Month><Day>3</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2018</Year><Month>12</Month><Day>12</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">29965278</ArticleId><ArticleId IdType="doi">10.13227/j.hjkx.201701171</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>République populaire de Chine</li></country></list><tree><country name="République populaire de Chine"><noRegion><name sortKey="Wang, Hong" sort="Wang, Hong" uniqKey="Wang H" first="Hong" last="Wang">Hong Wang</name></noRegion><name sortKey="Bu, Yu Wei" sort="Bu, Yu Wei" uniqKey="Bu Y" first="Yu-Wei" last="Bu">Yu-Wei Bu</name><name sortKey="Lu, Ping" sort="Lu, Ping" uniqKey="Lu P" first="Ping" last="Lu">Ping Lu</name><name sortKey="Xia, Wen" sort="Xia, Wen" uniqKey="Xia W" first="Wen" last="Xia">Wen Xia</name><name sortKey="Yang, Hao" sort="Yang, Hao" uniqKey="Yang H" first="Hao" last="Yang">Hao Yang</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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